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Computer Simulation of Diffusion of Pb-Bi Eutectic in Liquid Sodium by Molecular Dynamics Method

[+] Author Affiliations
Yingxia Qi, Minoru Takahashi

Tokyo Institute of Technology, Tokyo, Japan

Paper No. ICONE10-22236, pp. 621-626; 6 pages
doi:10.1115/ICONE10-22236
From:
  • 10th International Conference on Nuclear Engineering
  • 10th International Conference on Nuclear Engineering, Volume 2
  • Arlington, Virginia, USA, April 14–18, 2002
  • Conference Sponsors: Nuclear Engineering Division
  • ISBN: 0-7918-3596-0 | eISBN: 0-7918-3589-8
  • Copyright © 2002 by ASME

abstract

Lead-bismuth eutectic is a potential candidate for coolant of secondary loops of sodium-cooled fast breeder reactors (FBR). The studies on the diffusion of liquid Pb-Bi in liquid Na are carried out corresponding to the case that liquid Pb-Bi leaks to liquid Na by accident. As the diffusion processes are the results of atomic motions, molecular dynamics method has been used to study the diffusion process. The self-diffusion coefficients of pure liquid Pb and Na, and liquid Pb-Bi are calculated and compared with ones by the empirical equations. The discrepancy between them could be eliminated by changing the densities of the liquids. The diffusion of lead-bismuth in sodium is simulated based on the changed densities under which the self-diffusion coefficients of individual liquid metals are close to those by the empirical equations. The simulation results show that the diffusion process of liquid Pb-Bi in liquid Na is a heat releasing process and the density of ternary liquid Na-Pb-Bi is higher than the average value of the densities of liquid Na and liquid Pb-Bi. It is also found that the diffusion coefficients of liquid Pb-Bi in liquid Na are much higher than their self-diffusion coefficients, indicating that liquid Pb-Bi are easy and quickly to diffuse in liquid Na. However, the diffusion coefficient of liquid Na is decreased due to the existence of liquid Pb-Bi, implying that liquid Na-Pb-Bi have a higher viscosity than that of pure liquid Na.

Copyright © 2002 by ASME

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